Source Publication
AIP Advances
Document Type
Article
Publication Date
4-2014
DOI
10.1063/1.4871482
Abstract
The Rayleigh-Taylor (RT) interfacial instability has been attributed to physical phenomenon in a wide variety of macroscopic systems, including black holes, laser generated plasmas, and thick fluids. However, evidence for its existence in the nanoscale is lacking. Here we first show theoretically that this instability can occur in films with thickness negligible compared to the capillary length when they are heated rapidly inside a bulk fluid. Pressure gradients developed in the evaporated fluid region produce large forces causing the instability. Experiments were performed by melting Au films inside glycerol fluid by nanosecond laser pulses. The ensuingnanoparticles had highly monomodal size distributions. Importantly, the spacing of thenanoparticles was independent of the film thickness and could be tuned by the magnitude of the pressure gradients. Therefore, this instability can overcome some of the limitations of conventional thin self-organization techniques that rely on film thickness to control length scales.
Recommended Citation
Yadavali, S., and R. Kalyanaraman. "Nanomaterials Synthesis by a Novel Phenomenon: The Nanoscale Rayleigh-Taylor Instability." AIP Advances 4, no. 4 (2014). DOI: 10.1063/1.4871482.
Submission Type
Publisher's Version
Comments
This article was published openly thanks to the University of Tennessee Open Publishing Support Fund.
Licensed under a Creative Commons Attribution License (CC BY)