Masters Theses

Author

Yunnhon Lo

Date of Award

5-1996

Degree Type

Thesis

Degree Name

Master of Science

Major

Nuclear Engineering

Major Professor

Peter G. Groer

Committee Members

Laurence F. Miller, Lawrence W. Townsend

Abstract

The standard mathematical treatment of the build-up and decay of airborne radionuclides on a filter paper uses the solutions of the so-called Bateman equations adapted to the sampling process. These equations can be interpreted as differential equations for the expectation of an underlying stochastic process, which describes the random fluctuations in the accumulation and decay of the sampled radioactive atoms. The probability distribution for the number of 218Po, 214Pb and 214Bi atoms, accumulated after sampling time t, is the product of three Poisson distributions. We show that the distribution of the number of counts, registered by a detector with efficiency &epsilon during a counting period T after the end of sampling, is also the product of three Poisson distributions. Its mean is dependent on ε, t, T, flowrate, and N0A, N0B and N0C, the number of 218Po, 214Pb and 214Bi atoms per unit volume. This joint Poisson distribution was used to construct the likelihood given the observed number of counts. Using Bayes' Theorem we obtained posterior densities for N0A, N0B and N0C. These densities characterize the remaining uncertainty about the unknown airborne concentrations of 218Po, 214Pb and 214Bi atoms.

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