Doctoral Dissertations

Date of Award

3-1983

Degree Type

Dissertation

Degree Name

Doctor of Philosophy

Major

Chemistry

Major Professor

Earl L. Wehry

Committee Members

Lee Magid, Gleb Mamantov, Gary Sayler

Abstract

A solid, untreated solvent-refined coal sample yields matrix isolation fluorescence spectra suitable for the identification and determination of polycyclic aromatic hydrocarbons. Several PAHs can be identified in xenon-lamp excited spectra. The capability for selective excitation of fluorescence and background suppression using the time resolution of a dye-laser spectrometer permit the unambiguous identification of PAHs including benzo[a]pyrene. Quantitative "standard addition" plots for benzo[a]pyrene, perylene, benz[a]anthracene, and pyrene in SRC I are precise and appear to be reliable. Because of the absence of a suitable solid standard reference material, the accuracy of quantitative results cannot be ascertained.

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